The possibility of using push-pull systems based on furazanopyrazine in organic lightemitting diodes (OLEDs) and photovoltaic film devices was shown for the first time. The emission of all the obtained light-emitting diodes had a yellow-green color, and a maximum brightness of 45600 cd m-2 was achieved at a maximum current efficiency of 2.9 cd A-1. It was determined that the mobility of charge carriers measured in different current modes for these push-pull systems ranged from 10-4 to 4•10-6 cm2 V-1 s-1, considerably exceeding the values of the well-known compound Spiro-MeOTAD, widely used in high-efficiency photovoltaic devices.